You know, like films that are actually IN French or Spanish...
As above Pan's labyrinth, you could try The Orphanage and The Devils Backbone, all in Spanish, there's also a film Open Your Eyes/Abre Los Ojos which was remade in the English language as Vanilla Sky with Tom Cruise.
For French films, Amelie, La Femme Nikita. I've not seen them but the Three Colours trilogy is supposed to be very good (Three Colours Red, Blue White), and Diabolique (Les diaboliques) and Delicatessen is supposed to be very good (again I've not seen that one).
Sin Nombre is pretty good as is The Devil's Backbone. I've also recently recorded Cronos. If you want something a little light-hearted but emotional try Valentin. You should also have a look at any english DVDs you have as a lot of them will have a french or spanish language option =].
Have a look here too =] ---> http://funadvice.com/r/bt7ipgj5cpq
Women on the Brink of a Nervous Breakdown. Ma Vie en Rose (My Life in Pink). With a Friend Like Harry. Repulsion. Tomboy. Like Water for Chocolate. Amélie,
The long engagement. Priceless. The Valet. Jean De Florette. Manon of the Spring.(Don't want Manon without seeing Jean De Florette) Angela.
La Princesse de Montpensier :D and Sarah's Key. If you are interested in any good German films an excellent one was Im Juli.
Les miserables, Scarlet Pimpernel, Cyrano de Bergerac.
Pans labyrinth is really good