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What is collection of books called
It depends.
A library, yes - lots of different books, either available to the public (a public library) or not (a private library) a series - a set of books with a similar theme or even the same author (like the Nancy Drew detective series) an archive - like a library, a collection of printed materials (books but also other documents) (Most countries have National Archives, and most universities have their own archives as well)
a library?
a series